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Abstract Low-lying states in$$^{54}$$ $_{}^{54}$Cr have been investigated via the$$\alpha $$ $\alpha$-transfer reaction$$^{50}$$ $_{}^{50}$Ti($$^{7}$$ $_{}^7$Li,t) at a bombarding energy of 20 MeV. The exclusive$$\alpha $$ $\alpha$-transfer channel is separated from other reaction channels through the appropriate energy gate on the complementary particle, triton. Levels of$$^{54}$$ $_{}^{54}$Cr populated exclusively by the$$\alpha $$ $\alpha$-transfer process could be identified up to$$\approx $$ $\approx$5 MeV excitation energy and angular momentum up to$$(8)^{+}$$ ${\left(8\right)}^{+}$, by identifying the corresponding known$$\gamma $$ $\gamma$-rays. These include multiple low-lying non-yrast 2$$^+$$ $_{}^{+}$and 4$$^+$$ $_{}^{+}$states, which would otherwise be unfavorable via fusion evaporation reactions. The feeding-subtracted$$\gamma $$ $\gamma$-ray yields have been extracted to estimate the population of various excited states through the transfer process. The measured integrated transfer cross sections for all the observed yrast and non-yrast states are compared with Coupled Channels calculations usingfrescoto extract the$$\alpha $$ $\alpha$+$$^{50}$$ $_{}^{50}$Ti core spectroscopic factors. For the yrast states, a higher$$\alpha $$ $\alpha$+core overlap is seen for the$$2^+$$ $2^{+}$and$$4^+$$ $4^{+}$states, while it is seen to be less favorable for the$$6^+$$ $6^{+}$and$$(8)^+$$ ${\left(8\right)}^{+}$states when$$\alpha $$ $\alpha$-transfer is considered to occur predominantly as a direct one-step process to the$$^{50}$$ $_{}^{50}$Ti core ground state. The yrast$$2^+$$ $2^{+}$, and$$4^+$$ $4^{+}$states are predominantly populated by single-step transfer, while for the states with spin$$\ge $$ $\ge$5, the possibility of core excitation followed by$$\alpha $$ $\alpha$-transfer shows a larger$$\alpha $$ $\alpha$-core overlap. For the non-yrast$$0^+$$ $0^{+}$,$$2^+$$ $2^{+}$, and$$4^+$$ $4^{+}$states, single-step transfer shows moderate to small$$\alpha $$ $\alpha$-core overlap. No higher spin non-yrast states are observed.